首页> 外文OA文献 >Self-Propelled Colloidal Particle Near a Planar Wall: A Brownian Dynamics Study
【2h】

Self-Propelled Colloidal Particle Near a Planar Wall: A Brownian Dynamics Study

机译:平面墙附近的自行胶体粒子:布朗   动力学研究

代理获取
本网站仅为用户提供外文OA文献查询和代理获取服务,本网站没有原文。下单后我们将采用程序或人工为您竭诚获取高质量的原文,但由于OA文献来源多样且变更频繁,仍可能出现获取不到、文献不完整或与标题不符等情况,如果获取不到我们将提供退款服务。请知悉。

摘要

Miniaturized, self-propelled locomotors use chemo-mechanical transductionmechanisms to convert fuel in the environment to autonomous motion. Recentexperimental and theoretical studies demonstrate that these autonomous enginescan passively follow the contours of solid boundaries they encounter. Boundaryguidance, however, is not necessarily stable: Mechanical disturbances can causethe motor to hydrodynamically depart from the passively guided pathway.Furthermore, given the scaled-down size of micromotors (typically 100 nm -10$\mu$m), Brownian thermal fluctuation forces are necessarily important andthese stochastic forces can randomize passively-steered trajectories. Here we examine theoretically the stability of boundary guided motion ofmicromotors along infinite planar walls to mechanical disturbances and toBrownian forces. Our aim is to understand under what conditions this passivelyguided motion is stable. We choose a locomotor design in which sphericalcolloids are partially coated with a catalytic cap that reacts with solute toproduce a product. The product is repelled from the particle surface, causingthe particle to move with the inert face at the front (autonomous motion viaself-diffusiophoresis). When propelled towards a planar wall, deterministichydrodynamic studies demonstrate that these locomotors can exhibit, for largeenough cap sizes, steady trajectories in which the particle either skimsunidirectionally along the surface at a constant distance from the wall, orbecomes stationary. We first investigate the linear hydrodynamic stability ofthese states by expanding the equations of motion about the states, and findthat linear perturbations decay exponentially in time. We then study theeffects of thermal fluctuations by formulating a Langevin equation for theparticle motion which includes the Brownian stochastic force...
机译:小型化,自推进式机车使用化学机械转导机制将环境中的燃料转换为自主运动。最近的实验和理论研究表明,这些自主引擎可以被动地跟随它们遇到的实体边界的轮廓。然而,边界引导不一定是稳定的:机械干扰会导致电动机从流体动力学上脱离被动引导路径;此外,鉴于微型电动机的尺寸已缩小(通常为100 nm-10μm),布朗热波动力必不可少,这些随机力可以使被动转向的轨迹随机化。在这里,我们从理论上研究了微电机沿无限平面壁的边界引导运动对机械干扰和布朗力的稳定性。我们的目的是了解这种被动引导运动在什么条件下是稳定的。我们选择一种运动设计,其中球形胶体部分涂有催化帽,该催化帽与溶质反应生成产物。产物从颗粒表面被排斥,导致颗粒以惰性面朝前移动(通过自扩散电泳进行自主运动)。当被推向平坦的墙壁时,确定性的水动力研究表明,对于较大的瓶盖尺寸,这些运动电机可以表现出稳定的轨迹,其中粒子要么沿着表面以恒定的距离沿壁单向掠过,要么变为静止。我们首先通过扩展关于状态的运动方程来研究这些状态的线性流体动力稳定性,并发现线性扰动随时间呈指数衰减。然后,我们通过为粒子运动公式化Langevin方程来研究热涨落的影响,其中包括布朗随机力...

著录项

相似文献

  • 外文文献
  • 中文文献
  • 专利
代理获取

客服邮箱:kefu@zhangqiaokeyan.com

京公网安备:11010802029741号 ICP备案号:京ICP备15016152号-6 六维联合信息科技 (北京) 有限公司©版权所有
  • 客服微信

  • 服务号